| Id |
Subject |
Object |
Predicate |
Lexical cue |
| T1 |
0-144 |
Sentence |
denotes |
The source and characteristics of chemiluminescence associated with the oxygenase reaction catalyzed by Mn(2+)-ribulosebisphosphate carboxylase. |
| T2 |
145-224 |
Sentence |
denotes |
We confirm the observation of Mogel and McFadden (Mogel, S.N., and McFadden, B. |
| T3 |
225-412 |
Sentence |
denotes |
A. (1990) Biochemistry 29, 8333-8337) that ribulosebisphosphate carboxylase/oxygenase (rubisco) exhibits chemiluminescence while catalyzing its oxygenase reaction in the presence of Mn2+. |
| T4 |
413-527 |
Sentence |
denotes |
However, our results with the spinach and Rhodospirillum rubrum enzymes differ markedly in the following respects. |
| T5 |
528-672 |
Sentence |
denotes |
1) Chemiluminescence intensity was directly proportional to enzyme concentration and behaved as if representing the rate of oxygenase catalysis. |
| T6 |
673-750 |
Sentence |
denotes |
2) The wavelength spectrum peaked at about 770 nm and extended beyond 810 nm. |
| T7 |
751-863 |
Sentence |
denotes |
This seems inconsistent with chemiluminescence generated by simultaneous decay of pairs of singlet O2 molecules. |
| T8 |
864-949 |
Sentence |
denotes |
It is consistent with manganese(II) luminescence and we discuss its possible sources. |
| T9 |
950-1388 |
Sentence |
denotes |
The time course of chemiluminescence (resolution, 0.25 s) was distinctively different for spinach and R. rubrum enzymes during the initial 5 s of catalysis, with the bacterial enzyme exhibiting a pronounced initial "burst." Chemiluminescence by the spinach enzyme responded to substrate concentrations in a manner consistent with known oxygenase properties, exhibiting Michaelis-Menten kinetics with ribulose-1,5-bisphosphate (Km 400 nM). |
| T10 |
1389-1507 |
Sentence |
denotes |
Chemiluminescence required carbamylated enzyme with Mn2+ bound at the active site (activation energy, -57.1 KJ.mol-1). |
| T11 |
1508-1686 |
Sentence |
denotes |
As an indicator of oxygenase activity, chemiluminescence represents an improvement over oxygen electrode measurements in response time and sensitivity by factors of at least 100. |
| T1 |
0-144 |
Sentence |
denotes |
The source and characteristics of chemiluminescence associated with the oxygenase reaction catalyzed by Mn(2+)-ribulosebisphosphate carboxylase. |
| T2 |
145-224 |
Sentence |
denotes |
We confirm the observation of Mogel and McFadden (Mogel, S.N., and McFadden, B. |
| T3 |
225-412 |
Sentence |
denotes |
A. (1990) Biochemistry 29, 8333-8337) that ribulosebisphosphate carboxylase/oxygenase (rubisco) exhibits chemiluminescence while catalyzing its oxygenase reaction in the presence of Mn2+. |
| T4 |
413-527 |
Sentence |
denotes |
However, our results with the spinach and Rhodospirillum rubrum enzymes differ markedly in the following respects. |
| T5 |
528-672 |
Sentence |
denotes |
1) Chemiluminescence intensity was directly proportional to enzyme concentration and behaved as if representing the rate of oxygenase catalysis. |
| T6 |
673-750 |
Sentence |
denotes |
2) The wavelength spectrum peaked at about 770 nm and extended beyond 810 nm. |
| T7 |
751-863 |
Sentence |
denotes |
This seems inconsistent with chemiluminescence generated by simultaneous decay of pairs of singlet O2 molecules. |
| T8 |
864-949 |
Sentence |
denotes |
It is consistent with manganese(II) luminescence and we discuss its possible sources. |
| T9 |
950-1388 |
Sentence |
denotes |
The time course of chemiluminescence (resolution, 0.25 s) was distinctively different for spinach and R. rubrum enzymes during the initial 5 s of catalysis, with the bacterial enzyme exhibiting a pronounced initial "burst." Chemiluminescence by the spinach enzyme responded to substrate concentrations in a manner consistent with known oxygenase properties, exhibiting Michaelis-Menten kinetics with ribulose-1,5-bisphosphate (Km 400 nM). |
| T10 |
1389-1507 |
Sentence |
denotes |
Chemiluminescence required carbamylated enzyme with Mn2+ bound at the active site (activation energy, -57.1 KJ.mol-1). |
| T11 |
1508-1686 |
Sentence |
denotes |
As an indicator of oxygenase activity, chemiluminescence represents an improvement over oxygen electrode measurements in response time and sensitivity by factors of at least 100. |