PMC:7291971 / 77167-79205
Annnotations
LitCovid-PMC-OGER-BB
Id | Subject | Object | Predicate | Lexical cue |
---|---|---|---|---|
T1530 | 46-48 | CHEBI:30756;CHEBI:30756 | denotes | 9H |
T1531 | 49-59 | CHEBI:30756;CHEBI:30756 | denotes | purin-9-yl |
T1532 | 60-84 | CHEBI:53233;CHEBI:53233 | denotes | -2,2-dimethyl-tetrahydro |
T1533 | 85-87 | CHEBI:53233;CHEBI:53233 | denotes | 2H |
T1534 | 103-114 | CHEBI:86228;CHEBI:86228 | denotes | 3]dioxol-4- |
T1535 | 114-117 | CHEBI:53233;CHEBI:53233 | denotes | yl] |
T1536 | 117-123 | CHEBI:29309;CHEBI:29309 | denotes | methyl |
T1537 | 126-128 | CHEBI:86228;CHEBI:86228 | denotes | 4- |
T1538 | 128-134 | CHEBI:47853;CHEBI:47853 | denotes | chloro |
T1539 | 134-149 | CHEBI:86228;CHEBI:86228 | denotes | -3-nitrophenyl) |
T1540 | 149-155 | CHEBI:29309;CHEBI:29309 | denotes | methyl |
T1541 | 155-156 | CHEBI:86228;CHEBI:86228 | denotes | ] |
T1542 | 156-161 | CHEBI:46882;CHEBI:46882 | denotes | amino |
T1543 | 162-168 | CHEBI:42241;CHEBI:42241 | denotes | ethoxy |
T1544 | 170-171 | CHEBI:86228;CHEBI:86228 | denotes | 4 |
T1545 | 178-179 | CHEBI:53233;CHEBI:53233 | denotes | - |
T1546 | 179-197 | CHEBI:28714;CHEBI:28714 | denotes | butyldimethylsilyl |
T1547 | 197-198 | CHEBI:53233;CHEBI:53233 | denotes | ) |
T1548 | 198-201 | CHEBI:29354;CHEBI:29354 | denotes | oxy |
T1549 | 202-213 | CHEBI:53233;CHEBI:53233 | denotes | -5-{[(tert- |
T1550 | 213-231 | CHEBI:28714;CHEBI:28714 | denotes | butyldimethylsilyl |
T1551 | 231-232 | CHEBI:53233;CHEBI:53233 | denotes | ) |
T1552 | 232-235 | CHEBI:29354;CHEBI:29354 | denotes | oxy |
T1553 | 236-242 | CHEBI:16625;CHEBI:16625 | denotes | methyl |
T1554 | 243-255 | CHEBI:53233;CHEBI:53233 | denotes | oxolan-2-yl] |
T1555 | 256-258 | CHEBI:29238;CHEBI:29238 | denotes | 9H |
T1556 | 259-264 | CHEBI:17939;CHEBI:17939 | denotes | purin |
T1557 | 264-267 | CHEBI:17369;CHEBI:17369 | denotes | -6- |
T1558 | 267-272 | CHEBI:32952;CHEBI:32952 | denotes | amine |
T1559 | 283-291 | CHEBI:75958;CHEBI:75958 | denotes | solution |
T1560 | 365-373 | CHEBI:75958;CHEBI:75958 | denotes | solution |
T1561 | 377-379 | CHEBI:86228;CHEBI:86228 | denotes | 4- |
T1562 | 379-385 | CHEBI:47853;CHEBI:47853 | denotes | chloro |
T1563 | 385-406 | CHEBI:86228;CHEBI:86228 | denotes | -3-nitrobenazaldehyde |
T1564 | 465-476 | CHEBI:15366;CHEBI:15366 | denotes | acetic acid |
T1565 | 554-560 | CHEBI:35607;CHEBI:35607 | denotes | sodium |
T1566 | 561-582 | CHEBI:28621;CHEBI:28621 | denotes | triacetoxyborohydride |
T1567 | 660-668 | CHEBI:75958;CHEBI:75958 | denotes | solution |
T1568 | 724-731 | CHEBI:15377;CHEBI:15377 | denotes | aqueous |
T1569 | 732-738 | CHEBI:32139;CHEBI:32139 | denotes | NaHCO3 |
T1570 | 744-751 | CHEBI:15377;CHEBI:15377 | denotes | aqueous |
T1571 | 870-876 | CHEBI:34683;CHEBI:34683 | denotes | Na2SO4 |
T1572 | 965-971 | CHEBI:30563;CHEBI:30563 | denotes | silica |
T1573 | 998-1002 | CHEBI:32145;CHEBI:32145 | denotes | MeOH |
T1574 | 1063-1067 | CHEBI:32145;CHEBI:32145 | denotes | MeOH |
T1575 | 1096-1101 | CHEBI:30808;CHEBI:30808 | denotes | CDCl3 |
T1576 | 1676-1679 | CHEBI:36927;CHEBI:36927 | denotes | 13C |
T22187 | 46-48 | CHEBI:30756;CHEBI:30756 | denotes | 9H |
T61490 | 49-59 | CHEBI:30756;CHEBI:30756 | denotes | purin-9-yl |
T33609 | 60-84 | CHEBI:53233;CHEBI:53233 | denotes | -2,2-dimethyl-tetrahydro |
T72503 | 85-87 | CHEBI:53233;CHEBI:53233 | denotes | 2H |
T84826 | 103-114 | CHEBI:86228;CHEBI:86228 | denotes | 3]dioxol-4- |
T77669 | 114-117 | CHEBI:53233;CHEBI:53233 | denotes | yl] |
T74326 | 117-123 | CHEBI:29309;CHEBI:29309 | denotes | methyl |
T68910 | 126-128 | CHEBI:86228;CHEBI:86228 | denotes | 4- |
T29834 | 128-134 | CHEBI:47853;CHEBI:47853 | denotes | chloro |
T61527 | 134-149 | CHEBI:86228;CHEBI:86228 | denotes | -3-nitrophenyl) |
T2636 | 149-155 | CHEBI:29309;CHEBI:29309 | denotes | methyl |
T77144 | 155-156 | CHEBI:86228;CHEBI:86228 | denotes | ] |
T5108 | 156-161 | CHEBI:46882;CHEBI:46882 | denotes | amino |
T26563 | 162-168 | CHEBI:42241;CHEBI:42241 | denotes | ethoxy |
T54685 | 170-171 | CHEBI:86228;CHEBI:86228 | denotes | 4 |
T28095 | 178-179 | CHEBI:53233;CHEBI:53233 | denotes | - |
T7577 | 179-197 | CHEBI:28714;CHEBI:28714 | denotes | butyldimethylsilyl |
T76522 | 197-198 | CHEBI:53233;CHEBI:53233 | denotes | ) |
T62588 | 198-201 | CHEBI:29354;CHEBI:29354 | denotes | oxy |
T93366 | 202-213 | CHEBI:53233;CHEBI:53233 | denotes | -5-{[(tert- |
T84385 | 213-231 | CHEBI:28714;CHEBI:28714 | denotes | butyldimethylsilyl |
T90566 | 231-232 | CHEBI:53233;CHEBI:53233 | denotes | ) |
T91292 | 232-235 | CHEBI:29354;CHEBI:29354 | denotes | oxy |
T24654 | 236-242 | CHEBI:16625;CHEBI:16625 | denotes | methyl |
T77065 | 243-255 | CHEBI:53233;CHEBI:53233 | denotes | oxolan-2-yl] |
T32349 | 256-258 | CHEBI:29238;CHEBI:29238 | denotes | 9H |
T22971 | 259-264 | CHEBI:17939;CHEBI:17939 | denotes | purin |
T77363 | 264-267 | CHEBI:17369;CHEBI:17369 | denotes | -6- |
T35102 | 267-272 | CHEBI:32952;CHEBI:32952 | denotes | amine |
T87653 | 283-291 | CHEBI:75958;CHEBI:75958 | denotes | solution |
T87411 | 365-373 | CHEBI:75958;CHEBI:75958 | denotes | solution |
T67786 | 377-379 | CHEBI:86228;CHEBI:86228 | denotes | 4- |
T2415 | 379-385 | CHEBI:47853;CHEBI:47853 | denotes | chloro |
T47993 | 385-406 | CHEBI:86228;CHEBI:86228 | denotes | -3-nitrobenazaldehyde |
T2831 | 465-476 | CHEBI:15366;CHEBI:15366 | denotes | acetic acid |
T81538 | 554-560 | CHEBI:35607;CHEBI:35607 | denotes | sodium |
T68096 | 561-582 | CHEBI:28621;CHEBI:28621 | denotes | triacetoxyborohydride |
T17174 | 660-668 | CHEBI:75958;CHEBI:75958 | denotes | solution |
T52438 | 724-731 | CHEBI:15377;CHEBI:15377 | denotes | aqueous |
T1797 | 732-738 | CHEBI:32139;CHEBI:32139 | denotes | NaHCO3 |
T62375 | 744-751 | CHEBI:15377;CHEBI:15377 | denotes | aqueous |
T33887 | 870-876 | CHEBI:34683;CHEBI:34683 | denotes | Na2SO4 |
T87343 | 965-971 | CHEBI:30563;CHEBI:30563 | denotes | silica |
T10295 | 998-1002 | CHEBI:32145;CHEBI:32145 | denotes | MeOH |
T78188 | 1063-1067 | CHEBI:32145;CHEBI:32145 | denotes | MeOH |
T12440 | 1096-1101 | CHEBI:30808;CHEBI:30808 | denotes | CDCl3 |
T3563 | 1676-1679 | CHEBI:36927;CHEBI:36927 | denotes | 13C |
LitCovid-PubTator
Id | Subject | Object | Predicate | Lexical cue | tao:has_database_id |
---|---|---|---|---|---|
1446 | 340-343 | Chemical | denotes | DCE | |
1447 | 377-406 | Chemical | denotes | 4-chloro-3-nitrobenazaldehyde | |
1448 | 448-451 | Chemical | denotes | DCE | |
1449 | 465-476 | Chemical | denotes | acetic acid | MESH:D019342 |
1450 | 547-552 | Chemical | denotes | argon | MESH:D001128 |
1451 | 554-582 | Chemical | denotes | sodium triacetoxyborohydride | |
1452 | 686-689 | Chemical | denotes | DCM | |
1453 | 732-738 | Chemical | denotes | NaHCO3 | MESH:D017693 |
1454 | 777-780 | Chemical | denotes | DCM | |
1455 | 844-849 | Chemical | denotes | brine | MESH:C017082 |
1456 | 870-876 | Chemical | denotes | Na2SO4 | |
1457 | 965-975 | Chemical | denotes | silica gel | MESH:D058428 |
1458 | 998-1002 | Chemical | denotes | MeOH | |
1459 | 1006-1009 | Chemical | denotes | DCM | |
1460 | 1063-1067 | Chemical | denotes | MeOH | |
1461 | 1068-1071 | Chemical | denotes | DCM | |
1462 | 1079-1081 | Chemical | denotes | 1H | |
1463 | 1096-1101 | Chemical | denotes | CDCl3 | |
1464 | 1114-1116 | Chemical | denotes | 1H | |
1465 | 1128-1130 | Chemical | denotes | 1H | |
1466 | 1142-1144 | Chemical | denotes | 1H | |
1467 | 1160-1162 | Chemical | denotes | 2H | MESH:D003903 |
1468 | 1179-1181 | Chemical | denotes | 2H | MESH:D003903 |
1469 | 1197-1199 | Chemical | denotes | 2H | MESH:D003903 |
1470 | 1987-2003 | Chemical | denotes | C44H66N12O9Si2Cl | |
1471 | 1960-1964 | Disease | denotes | HRMS |
LitCovid-PD-CLO
Id | Subject | Object | Predicate | Lexical cue |
---|---|---|---|---|
T411 | 274-276 | http://purl.obolibrary.org/obo/CLO_0001000 | denotes | 35 |
T412 | 281-282 | http://purl.obolibrary.org/obo/CLO_0001020 | denotes | a |
T413 | 363-364 | http://purl.obolibrary.org/obo/CLO_0001020 | denotes | a |
T414 | 408-410 | http://purl.obolibrary.org/obo/CLO_0050509 | denotes | 27 |
T415 | 810-817 | http://purl.obolibrary.org/obo/OBI_0100026 | denotes | organic |
T416 | 810-817 | http://purl.obolibrary.org/obo/UBERON_0000468 | denotes | organic |
T417 | 1019-1021 | http://purl.obolibrary.org/obo/CLO_0001000 | denotes | 35 |
T418 | 1025-1026 | http://purl.obolibrary.org/obo/CLO_0001020 | denotes | a |
T419 | 2005-2008 | http://purl.obolibrary.org/obo/CLO_0007706 | denotes | M+H |
LitCovid-PD-CHEBI
Id | Subject | Object | Predicate | Lexical cue | chebi_id |
---|---|---|---|---|---|
T99640 | 38-59 | Chemical | denotes | 6-amino-9H-purin-9-yl | http://purl.obolibrary.org/obo/CHEBI_30756 |
T29293 | 40-45 | Chemical | denotes | amino | http://purl.obolibrary.org/obo/CHEBI_46882 |
T82586 | 65-73 | Chemical | denotes | dimethyl | http://purl.obolibrary.org/obo/CHEBI_33601|http://purl.obolibrary.org/obo/CHEBI_42266 |
T44634 | 117-123 | Chemical | denotes | methyl | http://purl.obolibrary.org/obo/CHEBI_32875|http://purl.obolibrary.org/obo/CHEBI_29309 |
T38253 | 128-134 | Chemical | denotes | chloro | http://purl.obolibrary.org/obo/CHEBI_47853 |
T59769 | 149-155 | Chemical | denotes | methyl | http://purl.obolibrary.org/obo/CHEBI_32875|http://purl.obolibrary.org/obo/CHEBI_29309 |
T51490 | 156-161 | Chemical | denotes | amino | http://purl.obolibrary.org/obo/CHEBI_46882 |
T70758 | 162-168 | Chemical | denotes | ethoxy | http://purl.obolibrary.org/obo/CHEBI_42241 |
T748 | 198-201 | Chemical | denotes | oxy | http://purl.obolibrary.org/obo/CHEBI_29354 |
T35101 | 232-235 | Chemical | denotes | oxy | http://purl.obolibrary.org/obo/CHEBI_29354 |
T750 | 236-242 | Chemical | denotes | methyl | http://purl.obolibrary.org/obo/CHEBI_32875|http://purl.obolibrary.org/obo/CHEBI_29309 |
T56159 | 256-272 | Chemical | denotes | 9H-purin-6-amine | http://purl.obolibrary.org/obo/CHEBI_16708 |
T40430 | 267-272 | Chemical | denotes | amine | http://purl.obolibrary.org/obo/CHEBI_32952 |
T54842 | 283-291 | Chemical | denotes | solution | http://purl.obolibrary.org/obo/CHEBI_75958 |
T87374 | 340-343 | Chemical | denotes | DCE | http://purl.obolibrary.org/obo/CHEBI_27789 |
T756 | 365-373 | Chemical | denotes | solution | http://purl.obolibrary.org/obo/CHEBI_75958 |
T74109 | 379-385 | Chemical | denotes | chloro | http://purl.obolibrary.org/obo/CHEBI_47853 |
T5740 | 448-451 | Chemical | denotes | DCE | http://purl.obolibrary.org/obo/CHEBI_27789 |
T759 | 465-476 | Chemical | denotes | acetic acid | http://purl.obolibrary.org/obo/CHEBI_15366 |
T71199 | 472-476 | Chemical | denotes | acid | http://purl.obolibrary.org/obo/CHEBI_37527 |
T32586 | 547-552 | Chemical | denotes | argon | http://purl.obolibrary.org/obo/CHEBI_49475 |
T94488 | 554-560 | Chemical | denotes | sodium | http://purl.obolibrary.org/obo/CHEBI_26708 |
T52531 | 660-668 | Chemical | denotes | solution | http://purl.obolibrary.org/obo/CHEBI_75958 |
T68791 | 686-689 | Chemical | denotes | DCM | http://purl.obolibrary.org/obo/CHEBI_15767 |
T58335 | 732-738 | Chemical | denotes | NaHCO3 | http://purl.obolibrary.org/obo/CHEBI_32139 |
T85038 | 777-780 | Chemical | denotes | DCM | http://purl.obolibrary.org/obo/CHEBI_15767 |
T7488 | 870-876 | Chemical | denotes | Na2SO4 | http://purl.obolibrary.org/obo/CHEBI_32149 |
T90420 | 965-971 | Chemical | denotes | silica | http://purl.obolibrary.org/obo/CHEBI_30563 |
T12080 | 998-1002 | Chemical | denotes | MeOH | http://purl.obolibrary.org/obo/CHEBI_17790 |
T47925 | 1006-1009 | Chemical | denotes | DCM | http://purl.obolibrary.org/obo/CHEBI_15767 |
T16758 | 1054-1056 | Chemical | denotes | Rf | http://purl.obolibrary.org/obo/CHEBI_33346 |
T56935 | 1063-1067 | Chemical | denotes | MeOH | http://purl.obolibrary.org/obo/CHEBI_17790 |
T65073 | 1068-1071 | Chemical | denotes | DCM | http://purl.obolibrary.org/obo/CHEBI_15767 |
T92650 | 1079-1081 | Chemical | denotes | 1H | http://purl.obolibrary.org/obo/CHEBI_49637 |
T24482 | 1096-1101 | Chemical | denotes | CDCl3 | http://purl.obolibrary.org/obo/CHEBI_85365 |
T46322 | 1114-1116 | Chemical | denotes | 1H | http://purl.obolibrary.org/obo/CHEBI_49637 |
T60945 | 1128-1130 | Chemical | denotes | 1H | http://purl.obolibrary.org/obo/CHEBI_49637 |
T82601 | 1142-1144 | Chemical | denotes | 1H | http://purl.obolibrary.org/obo/CHEBI_49637 |
T95044 | 1241-1243 | Chemical | denotes | 1H | http://purl.obolibrary.org/obo/CHEBI_49637 |
T91404 | 1267-1269 | Chemical | denotes | 1H | http://purl.obolibrary.org/obo/CHEBI_49637 |
T68720 | 1306-1308 | Chemical | denotes | 1H | http://purl.obolibrary.org/obo/CHEBI_49637 |
T98770 | 1345-1347 | Chemical | denotes | 1H | http://purl.obolibrary.org/obo/CHEBI_49637 |
T97976 | 1371-1373 | Chemical | denotes | 1H | http://purl.obolibrary.org/obo/CHEBI_49637 |
T70613 | 1410-1412 | Chemical | denotes | 1H | http://purl.obolibrary.org/obo/CHEBI_49637 |
T67635 | 1436-1438 | Chemical | denotes | 1H | http://purl.obolibrary.org/obo/CHEBI_49637 |
T41136 | 1475-1477 | Chemical | denotes | 1H | http://purl.obolibrary.org/obo/CHEBI_49637 |
T38412 | 1515-1517 | Chemical | denotes | 1H | http://purl.obolibrary.org/obo/CHEBI_49637 |
T26872 | 1553-1555 | Chemical | denotes | 1H | http://purl.obolibrary.org/obo/CHEBI_49637 |
T56080 | 1694-1699 | Chemical | denotes | CDCl3 | http://purl.obolibrary.org/obo/CHEBI_85365 |
LitCovid-PD-HP
Id | Subject | Object | Predicate | Lexical cue | hp_id |
---|---|---|---|---|---|
T33 | 686-689 | Phenotype | denotes | DCM | http://purl.obolibrary.org/obo/HP_0001644 |
T34 | 777-780 | Phenotype | denotes | DCM | http://purl.obolibrary.org/obo/HP_0001644 |
T35 | 1006-1009 | Phenotype | denotes | DCM | http://purl.obolibrary.org/obo/HP_0001644 |
T36 | 1068-1071 | Phenotype | denotes | DCM | http://purl.obolibrary.org/obo/HP_0001644 |
LitCovid-sentences
Id | Subject | Object | Predicate | Lexical cue |
---|---|---|---|---|
T516 | 0-277 | Sentence | denotes | 4.1.35 9-[(2R,5R)-3-[2-({[(4R,6R)-6-(6-amino-9H-purin-9-yl)-2,2-dimethyl-tetrahydro-2H-furo[3,4-d] [1,3]dioxol-4-yl]methyl}[(4-chloro-3-nitrophenyl)methyl]amino)ethoxy]-4-[(tert-butyldimethylsilyl)oxy]-5-{[(tert-butyldimethylsilyl)oxy]methyl}oxolan-2-yl]-9H-purin-6-amine (35) |
T517 | 278-505 | Sentence | denotes | To a solution of 20 (100 mg, 0.12 mmol, 1.00 eq) in anhydrous DCE (3.5 mL) was added a solution of 4-chloro-3-nitrobenazaldehyde (27 mg, 0.18 mmol, 1.50 eq) in anhydrous DCE (3.5 mL) and acetic acid (10 μL, 0.18 mmol, 1.50 eq). |
T518 | 506-621 | Sentence | denotes | After stirring for 20 min at 40 °C under argon, sodium triacetoxyborohydride (38 mg, 0.18 mmol, 1.50 eq) was added. |
T519 | 622-739 | Sentence | denotes | After stirring at 40 °C for 16 h, the solution was diluted with DCM (30 mL) and washed with saturated aqueous NaHCO3. |
T520 | 740-907 | Sentence | denotes | The aqueous layer was extracted with DCM (3 × 30 mL) and the combined organic extracts were washed with brine (60 mL), dried over Na2SO4 and concentrated under vacuum. |
T521 | 908-1053 | Sentence | denotes | The residue was purified by flash column chromatography (silica gel, linear gradient 0–5% MeOH in DCM) to give 35 as a white solid (105 mg, 87%). |
T522 | 1054-1078 | Sentence | denotes | Rf 0.71 (MeOH/DCM 5:95). |
T523 | 1079-1675 | Sentence | denotes | 1H NMR (500 MHz, CDCl3) δ 8.27 (s, 1H), 8.18 (s, 1H), 8.15 (s, 1H), 7.82 (br. s, 2H), 7.29–7.27 (m, 2H), 6.22 (br. s, 2H), 6.20 (br. s, 2H), 6.10 (d, J = 3.6 Hz, 1H), 5.99 (d, J = 2.1 Hz, 1H), 5.37 (dd, J = 6.5 Hz, J = 2.1 Hz, 1H), 4.91 (dd, J = 6.5 Hz, J = 3.7 Hz, 1H), 4.48 (t, J = 5.1 Hz, 1H), 4.30 (td, J = 6.7 Hz, J = 3.6 Hz, 1H), 4.22 (t, J = 4.2 Hz, 1H), 4.07 (dt, J = 5.8 Hz, J = 3.0 Hz, 1H), 3.99 (dd, J = 11.5 Hz, J = 3.4 Hz, 1H), 3.81–3.72 (m, 2H), 3.71–3.66 (m, 1H), 3.65–3.61 (m, 2H), 2.90–2.70 (m, 4H), 1.57 (s, 3H), 1.36 (s, 3H), 0.92 (s, 9H), 0.86 (s, 9H), 0.14 – - 0.02 (m, 12H). |
T524 | 1676-1959 | Sentence | denotes | 13C NMR (125 MHz, CDCl3) δ 155.8, 155.7, 153.1, 153.0, 149.6, 149.0, 147.8, 140.6, 140.1, 139.3, 133.0, 131.4, 125.6, 125.2, 120.3, 120.1, 114.6, 90.8, 87.0, 85.7, 84.9, 84.0, 83.4, 82.8, 69.6, 69.3, 61.8, 58.2, 56.4, 53.5, 27.2, 26.2, 25.8, 25.4, 18.6, 18.2, −4.5, −4.7, −5.2, −5.3. |
T525 | 1960-2011 | Sentence | denotes | HRMS (ESI+): m/z calcd for C44H66N12O9Si2Cl [M+H]+: |
T526 | 2012-2028 | Sentence | denotes | 997.4297, found: |
T527 | 2029-2038 | Sentence | denotes | 997.4327. |